Paola Massari et al.Download PDFPatent Trials and Appeals BoardOct 23, 201913698608 - (D) (P.T.A.B. Oct. 23, 2019) Copy Citation UNITED STATES PATENT AND TRADEMARK OFFICE UNITED STATES DEPARTMENT OF COMMERCE United States Patent and Trademark Office Address: COMMISSIONER FOR PATENTS P.O. Box 1450 Alexandria, Virginia 22313-1450 www.uspto.gov APPLICATION NO. FILING DATE FIRST NAMED INVENTOR ATTORNEY DOCKET NO. CONFIRMATION NO. 13/698,608 12/12/2012 Paola Massari FE6606 4325 24114 7590 10/23/2019 LyondellBasell Industries Legal IP Department 1221 McKinney Street, Suite 700 LyondellBasell Tower Houston, TX 77010 EXAMINER KRYLOVA, IRINA ART UNIT PAPER NUMBER 1764 NOTIFICATION DATE DELIVERY MODE 10/23/2019 ELECTRONIC Please find below and/or attached an Office communication concerning this application or proceeding. The time period for reply, if any, is set in the attached communication. Notice of the Office communication was sent electronically on above-indicated "Notification Date" to the following e-mail address(es): legal-IP@lyondellbasell.com PTOL-90A (Rev. 04/07) UNITED STATES PATENT AND TRADEMARK OFFICE ____________________ BEFORE THE PATENT TRIAL AND APPEAL BOARD ____________________ Ex parte PAOLA MASSARI, MARCO CIARAFONI, and TIZIANA CAPUTO ____________________ Appeal 2018-008554 Application 13/698,608 Technology Center 1700 ____________________ Before JEFFREY B. ROBERTSON, BRIAN D. RANGE, and DEBRA L. DENNETT, Administrative Patent Judges. DENNETT, Administrative Patent Judge. DECISION ON APPEAL1 STATEMENT OF THE CASE Appellant2 appeals under 35 U.S.C. § 134(a) from a final rejection of claims 1, 5–8, and 10–16. We have jurisdiction under 35 U.S.C. § 6(b). We AFFIRM. 1 In our Decision, we refer to the Non-final Office Action dated May 19, 2017 (“Non-final Act.”); the Final Office Action dated October 12, 2017 (“Final Act.”); the Appeal Brief filed March 9, 2018 (“Appeal Br.”); and the Examiner’s Answer dated May 29, 2018 (“Ans.”). Appellant does not file a Reply Brief. 2 We use the word “Appellant” to refer to the applicant as defined by 37 C.F.R. § 1.42. Appellant identifies the real party in interest as Basell Poliolefine Italia, S.R.L. Appeal Br. 2. Appeal 2018-008554 Application 13/698,608 2 The invention relates to a propylene composition having what are said to be improved balance of mechanical properties and excellent physical properties. Spec. 1, ll. 8–11. The propylene polymer composition is said to be particularly suitable for production of injection molded articles and films, which requires good flexibility and softness combined with high impact strength and good transparency. Spec. 1, ll. 12–14. Claim 1 is reproduced below from the Claims Appendix of the Appeal Brief and illustrates the claimed subject matter: 1. A propylene polymer composition consisting essentially of: A) 70-94 wt. % of a propylene-ethylene copolymer comprising 3.1-4 wt. % of ethylene derived units; and B) 6-30 wt. % of a second propylene-ethylene copolymer that is completely soluble in xylene comprising 41-55 wt. % of ethylene derived units; wherein the propylene polymer composition has: (i) a melt flow rate of 0.1-5 g/10 min, measured at 230 °C with a load of 2.16 kg; (ii) an intrinsic viscosity of the fraction soluble in xylene at room temperature of 2-4 dl/g; (iii) a flexural modulus of 300-600 MPa; (iv) at least one melting peak in a temperature range of 140-150 °C as determined via differential scanning calorimetry (DSC); and (v) at least one additive selected from the group consisting of antioxidants, light stabilizers, nucleating agents, antiacids, colorants, fillers and combinations thereof. Appeal 2018-008554 Application 13/698,608 3 REFERENCES The Examiner relies on the following prior art in rejecting the claims on appeal: Leonard et al. (“Leonard”) US 5,326,639 July 5, 1994 Pitkanen et al. (“Pitkanen”) US 6,342,564 B1 Jan. 29, 2002 Braga et al. (“Braga”) US 6,673,855 B1 Jan. 6, 2004 Borealis Tech. Oy (“Borealis”) EP 1 661 935 A1 May 31, 2006 REJECTION The Examiner maintains the following rejections3: A. Claims 1, 6–8, and 10–16 under 35 U.S.C. § 102(a)(1) as anticipated by, or in the alternative, under 35 U.S.C. § 103(a) as obvious over Leonard as evidenced by Braga; B. Claims 1, 5–8, and 10–16 under 35 U.S.C. § 102(a)(1) as anticipated by, or in the alternative, under 35 U.S.C. § 103(a) as obvious over Pitkanen as evidenced by Braga; C. Claims 5–8 and 10–16 under 35 U.S.C. § 103(a) as obvious over Leonard in view of Borealis, as evidenced by Braga; D. Claims 1, 5–8, and 10–16 under 35 U.S.C. § 103(a) as obvious over Leonard in view of Braga; and E. Claims 1, 5–8, and 10–16 under 35 U.S.C. § 103(a) as obvious over Pitkanen in view of Braga. Final Act. 3–8. 3 Because this application was filed before the March 16, 2013, effective date of the America Invents Act, we refer to the pre-AIA version of the statute. Appeal 2018-008554 Application 13/698,608 4 OPINION Appellant argues the claims as a group. Appeal Br. 4–10. We select the sole independent claim, claim 1, as representative of the groups identified in Rejections A, B, D, and E. 37 C.F.R. § 41.37(c)(1)(iv). The claims in Rejection C do not include claim 1, therefore we select claim 5 as representative of this group. Rejection A: claims 1, 6–8, and 10–16 as anticipated by or obvious over Leonard, as evidenced by Braga With respect to claim 1, the Examiner finds that Leonard discloses a thermoplastic polymer composition comprising: (A) 60–85 parts of a copolymer with an alpha olefin having the formula H2C=CHR, where R is H, containing over 85 wt.% of propylene units, specifically propylene- ethylene copolymer having 95–98 wt.% of propylene and having intrinsic viscosity of 0.5–3 dl/g; (B) about 1 wt.% of a semi-crystalline linear copolymer of ethylene and propylene, having intrinsic viscosity of 1–3 dl/g; (C) 10–39 parts of a copolymer of propylene with 30–80 wt.% of the alpha- olefin having the above formula, preferably 40–75 wt.%, soluble in xylene at room temperature, specifically propylene-ethylene copolymer and having intrinsic viscosity of 1–3 dl/g; wherein the composition comprises flexural modulus of lower than 1000 MPa to 150 MPa, preferably 150–700 MPa, such as 500 MPa. Non-Final Act. 5. The Examiner finds that Leonard’s composition comprises components (A) and (C) as the major components, with (B) used in an amount of “about 1 wt.%,” which the Examiner finds may be less than 1 wt.%. Id. at 6. The Examiner construes “consisting essentially of” as equivalent to “comprising.” Id. at 7. The Examiner finds nothing of record Appeal 2018-008554 Application 13/698,608 5 to suggest that the addition of 1 wt.% or less of component (B) of Leonard affects the novel and/or basic characteristics of Leonard’s thermoplastic olefin polymer. Id. at 6. The Examiner finds that Leonard’s component (A) inherently comprises 2–5 wt.% of an alpha olefin having the formula H2C=CHR where R is H (i.e., ethylene units) because the propylene-ethylene copolymer has 95–98 wt.% of propylene units. Id. at 7. Regarding the claimed melt flow rate and intrinsic viscosity elements of the claim, the Examiner finds that Examples 5 and 6 of Leonard have melt flow rates of 1.3–4.5 g/10 min and intrinsic viscosities of 1.56–2.75 dl/g. Id. at 8. The Examiner finds that Leonard teaches component (C) is soluble in xylene at room temperature. Id. Claim 1 requires a second propylene- ethylene copolymer that is completely soluble in xylene. Appeal Br. 12 (Claims App.). The Examiner acknowledges that Leonard does not specify that component (C) as “completely soluble” in xylene, but finds that (i) component (C) is specified as being amorphous and soluble in xylene; (ii) elastomeric/amorphous properties, and thus the solubility in xylene, increases with increased content of ethylene units; (iii) component (C) of Leonard is 40–75 wt.% ethylene. Non-Final Act. 8. The Examiner finds that Leonard’s component (C) is substantially the same as the second propylene-ethylene copolymer of claim 1 (comprising 41–55 wt.% of ethylene derived units), thus inherently will be or is reasonably expected to be completely soluble in xylene at room temperature. Id. The Examiner finds that Braga provides evidence that propylene-ethylene copolymers having 20–60 wt.% of ethylene are completely soluble in xylene at 25°C. Id. (citing Braga 3:19–22). Appeal 2018-008554 Application 13/698,608 6 The Examiner finds that Leonard’s composition comprises 60–85 wt.% propylene-ethylene copolymer comprising 2–5 wt.% ethylene and 10– 39 wt.% copolymer of propylene with 40–75 wt.% ethylene units. Id. at 9. The Examiner acknowledges that Leonard does not explicitly recite a melting peak of the composition, but finds that (i) Leonard’s composition is substantially the same as that claimed (comprising two propylene-ethylene copolymers used in relative amounts and/or overlapping ranges to those claimed, with substantially the same and/or overlapping ranges of ethylene comonomer to those claimed); and (ii) the crystallinity of the polypropylene composition, and thus its melting points, depends on the relative amounts of propylene and ethylene units. Id. The Examiner determines that Leonard will inherently or reasonably be expected to have at least one melting peak in a temperature range of 140–150°C, as claimed. Id. The Examiner finds that here the claimed and prior art products are identical or substantially identical in structure or composition, or are produced by identical or substantially identical processes, therefore, a prima facie case of either anticipation or obviousness is established. Id. at 8 (citing In re Best, 562 F.2d 1252, 1255 (CCPA 1977). Appellant argues that the similarities of Leonard (as well as Braga, Pitkanen, and Borealis) to the claimed invention are neither suggested nor supported when reading the reference in its entirety. Appeal Br. 6. Appellant contends that Leonard disadvantageously requires polymeric compositions comprising three or more components, which the claimed two component propylene polymer beneficially avoids, as reflected by the “consisting essentially of” transitional phrase. Id. Appeal 2018-008554 Application 13/698,608 7 Appellant contends that a mixture of component A and component B do not intrinsically or necessarily have a viscosity that falls between the lower limit of component A’s contribution to the viscosity of a solution and component B’s contribution to the viscosity of a solution. Id. at 7. Appellant argues that the Examiner’s conclusion has no rationale or evidence in support. Id. Appellant argues that Leonard does not reduce the number of options available for arriving at the claimed invention to a finite number of solutions, particularly in view of the inherent unpredictability in the chemical arts. Id. at 8. According to Appellant, one of ordinary skill in the art would have numerous possible choices and combinations of polypropylene/polyethylene concentrations and processing conditions to arrive at the result produced by claim 1. Id. Appellant also contends that the claimed polypropylene compositions provide surprising benefits, including enhanced mechanical properties, including but not limited to improved flexibility and impact properties. Id. at 8–9. Appellant argues that Table 2 of the Specification shows Izod impact resistance of Examples 1 and 2 is improved by up to 20-fold compared to Comparative Example 1. Id. at 9. Appellant argues that such unexpected properties teach away from combining known elements. Id. We address Appellant’s arguments in the order in which they are raised. First, Appellant contends that the two component polymer composition of claim 1 “beneficially avoid[s]” the “disadvantage[]” of polymeric compositions comprising three or more components. See Appeal Br. 6. Appellant provides no reasoning or analysis of why two components Appeal 2018-008554 Application 13/698,608 8 are beneficial or three components are disadvantageous. See id., generally. Moreover, “consisting essentially of” limits the scope of a claim to the specified materials and “those that do not materially affect the basic and novel characteristic(s)” of the claimed invention (emphasis added). In re Herz, 537 F.2d 549, 551–52 (CCPA 1976); see also PPG Indus. v. Guardian Indus. Corp., 156 F.3d 1351, 1354 (Fed. Cir. 1998) (“By using the term ‘consisting essentially of,’ the drafter signals that the invention necessarily includes the listed ingredients and is open to unlisted ingredients that do not materially affect the basic and novel properties of the invention.”); In re Janakirama-Rao, 317 F.2d 951, 954 (CCPA 1963) (“The word ‘essentially’ [in the phrase ‘consisting essentially of’] opens the claims to the inclusion of ingredients which would not materially affect the basic and novel characteristics of appellant’s composition as defined in the balance of the claim, according to the applicable law.”). Appellant has the burden of showing the basic and novel characteristics of the claimed composition. In re De Lajarte, 337 F.2d 870, 874 (CCPA 1964). However, Appellant does not adequately refute the Examiner’s finding that the record fails to show that less than 1 wt.% of Leonard’s component (B) materially affects the basic and novel characteristics of Leonard’s polymer. In addition, we agree with the Examiner’s determination that Leonard’s component (B) may be considered to fall within claim 1’s required “at least one additive.” See Ans. 23–24. Second, Appellant argues that the intrinsic viscosity of a mixture of component A and component B is not intrinsically or necessarily a viscosity that falls between the lower limit of component A’s contribution to the viscosity of a solution and component B’s contribution to the viscosity of a Appeal 2018-008554 Application 13/698,608 9 solution. Appeal Br. 7. Claim 1 requires that the composition have “an intrinsic viscosity of the fraction soluble in xylene at room temperature of 2– 4 dl/g.” Id. at 12 (Claims App.). Leonard discloses that its component (C), which the Examiner finds is equivalent to component B of claim 1, has an intrinsic viscosity of from 1 to about 3 dl/g, substantially overlapping the claimed range. See Leonard 4:24–27. Anticipation may be established when there is a substantial overlap between the ranges disclosed in the prior art and recited in claims such that one of ordinary skill in the art could readily envisage the claimed range from the prior art range. Atlas Powder Co. v. IRECO, Inc., 190 F.3d 1342, 1345 (Fed. Cir. 1999) (Anticipation was presumed based on a substantial overlap between the claimed ranges of ingredients in an explosive composition and the ranges of the same disclosed in a prior art reference.). A prima facie case of obviousness typically exists when the ranges of a claimed composition overlap the ranges disclosed in the prior art. In re Harris, 409 F.3d 1339, 1341 (Fed. Cir. 2005). Accordingly, Appellant’s argument is not commensurate in scope with claim 1. Third, Appellant contends that Leonard (and Borealis) do not reduce the number of options available to one of ordinary skill in the art to a finite number of solutions. Appeal Br. 8. Where one is required to “merely throw[] metaphorical darts at a board” in hopes of arriving at a successful result, but “the prior art gave either no indication of which parameters were critical or no direction as to which of many possible choices is likely to be successful,” courts should reject “hindsight claims of obviousness.” In re Kubin, 561 F.3d 1351, 1359 (Fed. Cir. 2009) (quoting In re O’Farrell, 853 F.2d 894, 903 (Fed. Cir. 1988). However, in the case at bar, Leonard Appeal 2018-008554 Application 13/698,608 10 discloses ranges of components (A) and (C) that overlap the claimed ranges, leaving the skilled artisan to merely pursue “known options” from “a finite number of identified, predictable solutions.” See KSR Int’l Co. v. Teleflex Inc., 550 U.S. 398, 421 (2007). Appellant’s fourth argument is that the claimed invention provides “surprising benefits.” Appeal Br. 8–9. For surprising benefits (unexpected results) to be probative evidence of non-obviousness Appellant must at least establish: (1) “there actually is a difference between the results obtained through the claimed invention and those of the prior art, In re Klosak, 455 F.2d 1077, 59 CCPA 862 (1972); and (2) that the difference actually obtained would not have been expected by one skilled in the art at the time of invention, id.; In re D’Ancicco, 439 F.2d 1244, 58 CCPA 1057 (1971).” In re Freeman, 474 F.2d 1318, 1324 (CCPA 1973). Moreover, “when unexpected results are used as evidence of nonobviousness, the results must be shown to be unexpected compared with the closest prior art.” In re Baxter Travenol Labs., 952 F.2d 388, 392 (Fed. Cir. 1991). And “the burden of showing unexpected results rests on he who asserts them.” In re Klosak, 455 F.2d at 1080. Unexpected results must also be “commensurate in scope with the degree of protection sought by the [claims on appeal].” In re Harris, 409 F.3d 1339, 1344 (Fed. Cir. 2005); In re Grasselli, 713 F.2d 731, 743 (Fed. Cir. 1983) (It is well settled “that objective evidence of non- obviousness must be commensurate in scope with the claims which the evidence is offered to support.”). Appellant’s arguments fail to meet any of the requirements needed to show surprising and unexpected results that make claim 1 patentable over Leonard. Appellant provides attorney argument, but no evidence, that one Appeal 2018-008554 Application 13/698,608 11 of ordinary skill in the art would not have expected the results obtained. Appellant contends that the single comparative example tested in the Specification is “in accordance with the preferred embodiments of Leonard and Borealis,” but provides nothing more in support, thus does not meet its burden of proof. See Appeal Br. 9. Appellant compares only two examples to a single comparative example (see Spec. 11–12, Table 2), thus the evidence is not commensurate in scope with the breadth of claim 1. Moreover, Appellant fails to establish that there is an unexpected difference in properties between Comparative Example 1 and Examples 1 and 2. See Spec. 12. All three compositions tested have copolymer A content, copolymer B content falling with the claimed ranges. Spec. 12, Table 2. Comparative Example 1 has a melt flow rate and melting peak within the ranges recited in claim 1. Id. Flexural Modulus of Comparative Example 1 was not tested, and thus cannot be compared. Although the intrinsic viscosity of Comparative Example 1 of 1.58 dl/g is outside the claimed range of 2–4 dl/g (id.), the Specification indicates that the polymer composition is broadly from 1–4.5 dl/g, which includes the intrinsic viscosity of the composition in Comparative Example 1. Spec. 3, ll. 7–10. Accordingly, Appellant does not sufficiently demonstrate unexpected or surprising results. Finally, Appellant contends that at least Leonard and Borealis teach away from the claimed invention. See Appeal Br. 9. However, teaching away requires that a reference “criticize, discredit, or otherwise discourage the solution claimed” by Appellant. In re Fulton, 391 F.3d 1195, 1201 (Fed. Cir. 2004). Appellant identifies nothing in any of the cited references that Appeal 2018-008554 Application 13/698,608 12 “criticize(s), discredit(s), or otherwise discourage(s)” production of claim 1’s propylene polymer composition. We sustain the Examiner’s rejection of claim 1 for the reasons given above. For these same reasons, we sustain the rejection of claims 6–8 and 10–16 in accordance with 37 C.F.R. § 41.37(c)(1)(iv). Rejection B: claims 1, 5–8, and 10–16 as anticipated by or obvious over Pitkanen, as evidenced by Braga Appellant’s arguments directed to Pitkanen are (1) the alleged similarities of the teachings of Pitkanen (as well as Leonard, Braga, and Borealis) are not suggested or supported when reading the references in their entirety (Appeal Br. 7); (2) the claims’ requirement that component B is completely soluble in xylene is not possible with the significant, amorphous fraction of the composition disclosed in Pitkanen (id. at 8); (3) the claimed composition provides surprising benefits and unexpected properties (id. at 8–9). The Examiner finds that amorphous polymers are soluble in xylene at room temperature, thus Pitkanen’s component B will inherently be or reasonably be expected to be completely soluble in xylene. Ans. 24 (citing Pitkanen 3:3–4). The Examiner also finds that Pitkanen discloses that component B is alternatively “amorphous or semicrystalline/amorphous,” and “may” comprise a crystalline phase, thus would be reasonably expected to be completely soluble in xylene when free from the crystalline phase. Id. Other than a one-sentence assertion, Appellant provides no further analysis or explanation of why Pitkanen’s disclosure fails to teach the claimed composition. Appellant provides no counter argument to the Examiner’s finding that Pitkanen’s amorphous portion would be completely Appeal 2018-008554 Application 13/698,608 13 soluble in xylene. For reasons discussed supra, Appellant does not show surprising and unexpected results with the claimed composition. Appellant fails to show that the Examiner reversibly erred in rejecting claim 1 and the dependent claims as anticipated by or obvious over Pitkanen, as evidenced by Braga. Rejection C: claims 5–8, and 10–16 as obvious over Leonard in view of Borealis, as evidenced by Braga Claims 5–8 and 10–16 depend directly from claim 1. Appeal Br. 12– 13. We held claims 6–8 and 10–16 to be anticipated by and obvious over Leonard in Rejection A supra, therefore we need not address these claims further. Claim 5, not subject to the previous rejections, requires “[a] film comprising the propylene polymer composition of claim 1.” Id. at 12. The Examiner relies on the disclosures of Leonard as evidence by Braga discussed in relation to claim 1. Final Act. 6 (citing Non-Final Act. 22–24). The Examiner finds that Leonard does not explicitly disclose a film, but finds that Borealis teaches a composition and film, the composition having amounts of components A and B within the claimed ranges, and intrinsic viscosity of each of components A and B within the claimed range. Non-Final Act. 23. The Examiner determines that it would have been obvious to one of ordinary skill in the art to use Leonard’s composition for making films, as taught by Borealis, because both references teach propylene-ethylene copolymer compositions having low MRF and low intrinsic viscosity used for making molded articles, and the films produced comprise very good tear features. Id. at 24. Appellant does not address the Examiner’s finding regarding Borealis’s teaching of a film. See generally Appeal Br. Appellant argues Appeal 2018-008554 Application 13/698,608 14 that “both Leonard and Borealis disadvantageously require polymeric compositions comprising three or more components, which is beneficially avoided by the two component, [polypropylene] based composition of the [claimed] invention as reflected and clearly encompassed by the ‘consisting essentially of’ transitional phrase.” Appeal Br. 6. We addressed Appellant’s argument in relation to Rejection A supra. As stated, Appellant has the burden of showing the basic and novel characteristics of the claimed composition in order to demonstrate that three components are excluded by the claim. In re De Lajarte, 337 F.2d at 874. Appellant fails to adequately refute the Examiner’s finding. Appellant also contends that the Examiner has not provided any facts to support the assertion that the composition of Borealis would have the claimed intrinsic viscosity. Appeal Br. 7. In response, the Examiner cites to Borealis at paragraphs 5 and 20, which disclose intrinsic viscosity. Ans. 25. Appellant fails to reply to this finding. Appellant does not show reversible error in the Examiner’s rejection of claim 5. Rejection D: claims 1, 5–8, and 10–16 as obvious over Leonard in view of Braga Having found the claims to be anticipated by and obvious over Leonard supra, we need not address this rejection further. Rejection E: claims 1, 5–8, and 10–16 as obvious over Pitkanen in view of Braga Having found the claims to be anticipated by and obvious over Pitkanen supra, we need not address this rejection further. We sustain the Examiner’s rejections of claims 1, 5–8, and 10–16. Appeal 2018-008554 Application 13/698,608 15 CONCLUSION In summary: Claim(s) Rejected 35 U.S.C. § References(s)/Basis Affirmed Reversed 1, 6–8, 10– 16 102(a) or 103(a) Leonard, Braga 1, 6–8, 10– 16 1, 5–8, 10– 16 102(a) or 103(a) Pitkanen, Braga 1, 5–8, 10– 16 5–8, 10–16 103(a) Leonard, Borealis, Braga 5–8, 10–16 1, 5–8, 10– 16 103(a) Leonard, Braga 1, 5–8, 10– 16 1, 5–8, 10– 16 103(a) Pitkanen, Braga 1, 5–8, 10– 16 Overall Outcome 1, 5–8, 10– 16 No time period for taking any subsequent action in connection with this appeal may be extended under 37 C.F.R. § 1.136(a)(1)(iv). AFFIRMED Copy with citationCopy as parenthetical citation