Megan Donovan et al.Download PDFPatent Trials and Appeals BoardJul 29, 201913589219 - (D) (P.T.A.B. Jul. 29, 2019) Copy Citation UNITED STATES PATENT AND TRADEMARK OFFICE UNITED STATES DEPARTMENT OF COMMERCE United States Patent and Trademark Office Address: COMMISSIONER FOR PATENTS P.O. Box 1450 Alexandria, Virginia 22313-1450 www.uspto.gov APPLICATION NO. FILING DATE FIRST NAMED INVENTOR ATTORNEY DOCKET NO. CONFIRMATION NO. 13/589,219 08/20/2012 Megan DONOVAN 71470-US-NP 1013 14269 7590 07/29/2019 The Dow Chemical Company/Ronald Bakule P.O. BOX 1967 2040 Dow Center Midland, MI 48641 EXAMINER RIETH, STEPHEN EDWARD ART UNIT PAPER NUMBER 1764 NOTIFICATION DATE DELIVERY MODE 07/29/2019 ELECTRONIC Please find below and/or attached an Office communication concerning this application or proceeding. The time period for reply, if any, is set in the attached communication. Notice of the Office communication was sent electronically on above-indicated "Notification Date" to the following e-mail address(es): FFUIMPC@dow.com PTOL-90A (Rev. 04/07) UNITED STATES PATENT AND TRADEMARK OFFICE ____________ BEFORE THE PATENT TRIAL AND APPEAL BOARD ____________ Ex parte MEGAN DONOVAN, ALVIN M. MAURICE, EDWIN H. NUNGESSER, and WEI ZHANG ____________ Appeal 2018-005287 Application 13/589,219 Technology Center 1700 ____________ Before ROMULO H. DELMENDO, WESLEY B. DERRICK, and JANE E. INGLESE, Administrative Patent Judges. INGLESE, Administrative Patent Judge. DECISION ON APPEAL Appellants1 request our review under 35 U.S.C. § 134(a) of the Examiner’s decision to finally reject claims 1 and 3–52. We have jurisdiction over this appeal under 35 U.S.C. § 6(b). We AFFIRM. 1 Appellants identify DowDuPont as the real party in interest. Appeal Brief filed January 3, 2018 (“App. Br.”), 3. 2 Final Office Action entered June 7, 2017 (“Final Act.”), 1. Appeal 2018-005287 Application 13/589,219 2 STATEMENT OF THE CASE Claim 1, the sole pending independent claim, illustrates the subject matter on appeal, and is reproduced below with language italicized that is of particular relevance to the present appeal: 1. An aqueous composition consisting essentially of: a particulate polymer having a particle diameter of from 0.7 microns to 50 microns, said polymer comprising, as copolymerized units, from 0.3% to 1 %, by weight based on said polymer weight, monomer selected from the group consisting of styrene and alpha-methylstyrene, said polymer having been formed in the presence of from 0.01 % to 0.5% isoascorbic acid, by weight based on said polymer weight; said particulate polymer being denser than water; and from 0.1 % to 5%, by weight based on said polymer weight, thickener. App. Br. 12 (Claims Appendix) (emphasis added and spacing altered relative to original). The Examiner maintains the following rejections in the Examiner’s Answer entered February 28, 2018: I. Claims 1, 3, and 4 under 35 U.S.C. § 103(a) as unpatentable over Bardman3 as evidenced by Density of Polymers4; 3 Bardman et al., US 2007/0043162 A1, issued February 22, 2007 (“Bardman”). 4 SCIENTIFIC POLYMER PRODUCTS, INC., Density of Polymers (by density), http://scientificpolymer.com/density-of-polymers-by-density (“Density of Polymers”). Appeal 2018-005287 Application 13/589,219 3 II. Claim 5 under 35 U.S.C. § 103(a) as unpatentable over Bardman as evidenced by Specia1Chem4Coatings5 and Density of Polymers; and III. Claims 1 and 3–5 under 35 U.S.C. § 103(a) as unpatentable over Chiou6 as evidenced by Density of Polymers. DISCUSSION Upon consideration of the evidence relied upon in this appeal and each of Appellants’ contentions, we affirm the Examiner’s rejections of claims 1 and 3–5 under 35 U.S.C. § 103(a), for the reasons set forth in the Final Action, the Answer, and below. We review appealed rejections for reversible error based on the arguments and evidence the appellants provide for each issue the appellants identify. 37 C.F.R. § 41.37(c)(1)(iv); Ex parte Frye, 94 USPQ2d 1072, 1075 (BPAI 2010) (precedential) (cited with approval in In re Jung, 637 F.3d 1356, 1365 (Fed. Cir. 2011) (Explaining that even if the Examiner had failed to make a prima facie case, “it has long been the Board’s practice to require an applicant to identify the alleged error in the examiner’s rejections.”)). Rejection I: claims 1, 3, and 4 under 35 U.S.C. § 103(a) as unpatentable over Bardman as evidenced by Density of Polymers Appellants argue claims 1, 3, and 4 together, and, therefore, do not present arguments directed to the separate patentability of any particular 5 NATROSOL® 250 HR, www.specialchem4coatings.com/tds/natrosol-250- hr/ashland-inc/4979/index.aspx (“Specia1Chem4Coatings”). 6 Chiou et al., US 2007/0218291 A1, issued September 20, 2007 (“Chiou”). Appeal 2018-005287 Application 13/589,219 4 claim. App. Br. 6–7. We, accordingly, select claim 1 as representative, and decide the appeal as to claims 1, 3, and 4 based on claim 1 alone. 37 C.F.R. § 41.37(c)(1)(iv). Bardman discloses an aqueous dispersion of particles comprised of first and second polymers. Bardman ¶¶ 2, 5. Bardman discloses that the particles have an average diameter of from 0.2 to 1.5 microns. Id. ¶ 18. Bardman discloses that the polymeric particles comprise from 10% to 80% by weight of the first polymer, which Bardman indicates comprises at least one monoethylenically unsaturated monomer, and from 0.05% to 90% by weight of at least one multi-ethylenically unsaturated monomer. Id. ¶ 5. Bardman discloses that suitable ethylenically unsaturated monomers include styrene and substituted styrenes. Id. ¶ 7. Appellants do not dispute the Examiner’s determination that Bardman indicates from these disclosures that the first polymer comprises from 10% to 99.95% by weight of a monoethylenically unsaturated monomer, which, as discussed above, Bardman discloses can be styrene. Compare Final Act. 4, with App. Br. 6– 7. Nor do Appellants dispute the Examiner’s determination that because Bardman’s polymeric particles comprise from 10% to 80% by weight of the first polymer, the amount of styrene or substituted styrenes in Bardman’s polymeric particles would be 1% to 80% by weight, which overlaps the range recited in claim 1. Compare Final Act. 4, with App. Br. 6–7. The Examiner finds that Example 7 of Bardman describes preparing polymeric particles from a first polymer comprising styrene in a process that utilizes iso-ascorbic acid. Final Act. 4; see also Bardman ¶¶ 62, 67. Appellants argue that the range of styrene content in Bardman’s polymeric particles calculated by the Examiner—1 % to 80 %—overlaps the Appeal 2018-005287 Application 13/589,219 5 range recited in claim 1 (0.3% to 1%) by only “one point,” and Appellants assert that Bardman does not provide any “motivation” that would have led one of ordinary skill in the art to the “lower levels” recited in claim 1. App. Br. 6–7. It is well-established, however, that “[i]n cases involving overlapping ranges . . . even a slight overlap in range establishes a prima facie case of obviousness.” In re Peterson, 315 F.3d 1325, 1329–30 (Fed. Cir. 2003). As discussed below, Appellants do not demonstrate the criticality of the styrene or alpha-methylstyrene weight percentages recited in claim 1. Consequently, Appellants’ arguments are insufficient to rebut the prima facie case of obviousness established by the uncontroverted overlap between the styrene or alpha-methylstyrene weight range recited in claim 1 and the styrene or substituted styrene weight range implicitly disclosed in Bardman. In re Woodruff, 919 F.2d 1575, 1578 (Fed. Cir. 1990) (indicating that in cases in which the difference between the claimed invention and the prior art is some range or other variable within the claims, the applicant must show that the particular range is critical, generally by showing that the claimed range achieves unexpected results relative to the prior art range.). Appellants argue that only one stage of the polymer synthesis described in Bardman’s Example 7 occurs in the presence of a non- formaldehyde reductant, and Appellants argue that the Examiner’s conclusion that the exemplified particles are formed in presence of a non- formaldehyde reductant is, therefore, flawed. App. Br. 7; Reply Br. 2–3. Appellants argue that the Examiner does not point to any teaching or suggestion in Bardman indicating that “the reductant is in any manner critical.” App. Br. 7. Appeal 2018-005287 Application 13/589,219 6 The recitation in claim 1, however, of “said polymer having been formed in the presence of from 0.01% to 0.5% isoascorbic acid, by weight based on said polymer weight” is a product-by-process limitation. It is well- established that “even though product-by-process claims are limited by and defined by the process, determination of patentability is based on the product itself.” In re Thorpe, 777 F.2d 695, 697 (Fed. Cir. 1985). Accordingly, for a claim that includes a product-by-process limitation, once the examiner provides a rationale tending to show that the claimed product appears to be the same or similar to that of the prior art, although produced by a different process, the burden shifts to the appellants to come forward with evidence establishing an unobvious difference between the claimed product and the prior art product. In re Marosi, 710 F.2d 799, 802 (Fed. Cir. 1983). In the present case, Example 7 of Bardman describes preparing an aqueous dispersion of polymeric particles by a process that includes preparing a monomer emulsion from methyl(meth)acrylate and butyl acrylate, and combining the monomer emulsion with a first polymer comprising styrene (prepared as described in Bardman’s Example 2), t-butyl hydroperoxide, iso-ascorbic acid, and water. Bardman ¶¶ 62, 67. Although Example 2 of Bardman, which describes preparing the first polymer from styrene monomers, does not disclose forming the polymer in the presence of iso-ascorbic acid (id. ¶ 62), the Examiner determines that “it is unclear how or why the implied product structure would be any different should isoascorbic acid be used in one or all of the stages involved in polymerization.” Ans. 11–12. Thus, the Examiner sets forth a rationale tending to show that the particulate polymer recited in claim 1 appears to be the same or similar to the polymeric particles of Example 7 of Bardman. Appeal 2018-005287 Application 13/589,219 7 The burden, therefore, shifts to Appellants to come forward with evidence establishing an unobvious difference between the particulate polymer recited in claim 1 and the polymeric particles produced as described in Example 7 of Bardman. On the record before us, Appellants do not meet this burden. Specifically, Appellants do not provide any evidence establishing an unobvious difference between the polymeric particles produced as described in Example 7 of Bardman and particulate polymer recited in claim 1. App. Br. 6–8. Nor do Appellants establish that use of an isoascorbic acid reductant to produce a particulate polymer as recited in claim 1 would result in a particulate polymer that is structurally distinct or different from polymeric particles produced as described in Bardman’s Example 7. Id. Appellants argue that the size of the polymeric particles produced as described in Bardman’s Example 7 is 526 nm, which is outside the particle size range recited in claim 1, and Appellants contend that the particle size is “a critical factor in [A]ppellants’ invention to prevent sedimentation in their dispersions of particles.” App. Br. 7. Bardman’s disclosures are not limited to Example 7, however. As discussed above, Bardman broadly discloses polymeric particles having an average particle diameter of from 0.2 to 1.5 microns, which overlaps the particle size range recited in claim 1, rendering the recited range prima facie obvious. Peterson, 315 F.3d at 1329–30. On this appeal record, Appellants do not present any evidence establishing the criticality of the particle size range recited in claim 1. Appellants’ unsupported arguments to the contrary are, therefore, unpersuasive of reversible error in the Examiner’s rejection. Woodruff, 919 F.2d at 1578 (Fed. Cir. 1990); Icon Health & Fitness, Inc. v. Appeal 2018-005287 Application 13/589,219 8 Strava, Inc., 849 F.3d 1034, 1043 (Fed. Cir. 2017) (“Attorney argument is not evidence” and cannot rebut other admitted evidence). Appellants argue that “the essential element in Bardman” is that the particles disclosed in the reference “include structure that provides, when dry, at least one void,” and Appellants contend that “there is no basis for an obviousness rejection over Bardman absent a rationale within Bardman for eliminating this critical structural element or rendering it optional.” App. Br. 7. As the Examiner explains (Ans. 14), however, Bardman explicitly indicates that the polymeric particles described in the reference include at least on void when dry, while claim 1 recites an aqueous composition consisting essentially of a particulate polymer. Bardman ¶ 20. Moreover, as the Examiner also explains, claim 1 does not exclude voids from being present in the particulate polymer recited in the claim. Ans. 14. Although Appellants argue that Bardman is an “inappropriate” reference because “it is entirely directed to a different and unrelated objective” than Appellants’ invention (App. Br. 6), it is well-established that “[i]n determining whether the subject matter of a patent claim is obvious, neither the particular motivation nor the avowed purpose of the patentee controls.” KSR Int’l Co. v. Teleflex Inc., 550 U.S. 398, 419 (2007). Consequently, Appellants’ argument are unpersuasive of reversible error in the Examiner’s rejection of claims 1, 3, and 4 under 35 U.S.C. Appeal 2018-005287 Application 13/589,219 9 § 103(a) as unpatentable over Bardman as evidenced by Density of Polymers7, which we accordingly sustain. Rejection II: claim 5 under 35 U.S.C. § 103(a) as unpatentable over Bardman as evidenced by Specia1Chem4Coatings and Density of Polymers To address this rejection, Appellants rely on the arguments discussed above that Appellants present for Rejection I, and contend that the additional reference applied in this rejection fails to remedy the deficiencies of Bardman. App. Br. 8. Because we are unpersuaded of reversible error in the Examiner’s rejection of claim 1 for reasons discussed above, Appellants’ position as to this ground of rejection is also unpersuasive of reversible error. Rejection III: claims 1 and 3–5 under 35 U.S.C. § 103(a) as unpatentable over Chiou as evidenced by Density of Polymers Appellants argue claims 1 and 3–5 together, and, therefore, do not present arguments directed to the separate patentability of any particular claim. App. Br. 8–11. We, accordingly, select claim 1 as representative, and decide the appeal as to claims 1 and 3–5 based on claim 1 alone. 37 C.F.R. § 41.37(c)(1)(iv). Chiou discloses an aqueous coating composition comprising duller particles having an average diameter of 1 to 20 microns. Chiou ¶ 8. Chiou discloses that the duller particles may be comprised of multi-stage polymers having rubbery cores comprising copolymers that include one or more vinyl monomers, such as styrene, in an amount of from 0 to 50 % by weight. Id. 7 Because Appellants do not contest the Examiner’s reliance on Density of Polymers, we need not address this reference for disposition of this appeal. App. Br. 7. Appeal 2018-005287 Application 13/589,219 10 ¶¶ 35, 36. Chiou discloses that one or more shell polymers surround the core copolymers, and explains that the shell polymers comprise from about 0.1% to about 40% of the total particle weight. Id. ¶ 39. Appellants do not dispute the Examiner’s determination that Chiou implicitly indicates from these disclosures that the core copolymers constitute 60%–99.9% by weight of the particles. Compare Final Act. 8, with App. Br. 8–11. The Examiner determines that because Chiou discloses that the core copolymers can include 0 to 50% by weight styrene, Chiou describes embodiments in which duller particles include 0% to 30% by weight styrene. Final Act. 8. Chiou discloses producing the duller particles by an emulsion polymerization process that involves use of a redox initiator coupled with a reductant, such as isoascorbic acid. Chiou ¶¶ 64–67. Appellants argue that the styrene level in the three-stage polymer described in Chiou’s Example 1 is approximately 0.1 weight%, which is outside the range recited in claim 1, and “the styrene stage was not prepared in the presence of a reductant, much less isoscorbic acid.” App. Br. 9. Appellants argue that the Examiner’s determination that Chiou discloses particles that include 0% to 30% styrene “appears to [be] based on compositions from two different embodiments of the rubbery cores of duller particles A and the level of shell polymer in duller particles A.” Id. Although the styrene content of the particles described in Example 1 of Chiou may be outside the range recited in claim 1 as Appellants assert, Chiou’s disclosures are not limited to Example 1. Rather, as discussed above, Chiou more broadly discloses duller particles that may be comprised of multi-stage polymers having rubbery cores surrounded by one or more shell polymers. Contrary to Appellants’ arguments, the rubbery cores and Appeal 2018-005287 Application 13/589,219 11 shell polymers described in Chiou are not directed to different embodiments, but, rather, relate to different stages of multi-stage polymers that constitute the duller particles described in the reference. As also discussed above, Chiou indicates that the rubbery cores may comprise copolymers including one or more vinyl monomers, such as styrene, in an amount of from 0 to 50 % by weight, while the shell polymers comprise from about 0.1% to about 40% of the total particle weight. As the Examiner determines (Final Act. 8), because Chiou discloses that the shell polymers comprise from about 0.1% to about 40% of the total particle weight, Chiou implicitly indicates that the core copolymers constitute 60%–99.9% by weight of the particles. And as the Examiner also determines (Final Act. 8), because Chiou discloses that the rubbery cores may comprise copolymers that include 0 to 50 % by weight styrene monomers, Chiou implicitly discloses duller particles that may include 0 to 30 % by weight styrene monomers, which encompasses the styrene monomer range recited in claim 1. Furthermore, although the styrene-containing polymer of the three- stage polymer described in Chiou’s Example 1 may not have been prepared in the presence of isoscorbic acid as Appellants assert, we point out again that Chiou’s disclosures are not limited to Example 1. Rather, as discussed above, Chiou more broadly discloses producing the duller particles described in the reference by an emulsion polymerization process that involves use of a redox initiator coupled with a reductant, such as isoascorbic acid. In re Mercier, 515 F.2d 1161, 1165 (CCPA 1975) (“[A]ll of the relevant teachings of the cited references must be considered in determining what they fairly teach to one having ordinary skill in the art.”). Appeal 2018-005287 Application 13/589,219 12 Appellants argue that Chiou’s teaching that styrene is optional (due to the 0% lower weight limit) discourages any conclusion that styrene is beneficial to Chiou’s objective, “thereby negating the criticality of styrene,” and, therefore, “Chiou directs one skilled in the art away from experimenting with that monomer and closely related monomers,” and would not have motivated one skilled in the art towards styrene in the amount recited in claim 1. App. Br. 9–10. As discussed above, however, Chiou implicitly discloses duller particles that may include 0 to 30 % by weight styrene monomer, which encompasses the styrene monomer weight range recited in claim 1, rendering the recited range prima facie obvious. We find no disclosure in Chiou that criticizes or disparages use of styrene and closely related monomers in the polymeric particles described in the reference, and Appellants do not identify any such disclosure. App. Br. 8–11. Contrary to Appellants’ arguments, Chiou, therefore, would not have directed one of ordinary skill in the art away from particulate polymers having a styrene content as recited in claim 1. DyStar Textilfarben GmbH & Co. Deutschland KG v. C.H. Patrick Co., 464 F.3d 1356, 1364 (Fed. Cir. 2006) (“We will not read into a reference a teaching away from a process where no such language exists.”); In re Fulton, 391 F.3d 1195, 1201 (Fed. Cir. 2004) (“The prior art’s mere disclosure of more than one alternative does not constitute a teaching away from any of these alternatives because such disclosure does not criticize, discredit, or otherwise discourage the solution claimed”); In re Gurley, 27 F.3d 551, 552–53 (Fed. Cir. 1994). Appellants argue that Chiou “generically discloses a list of at least 21 formaldehyde and non-formaldehyde reducing agents . . . unconnected to Appeal 2018-005287 Application 13/589,219 13 any particular particle size, composition, or the like, or any functional result of a composition prepared therefrom.” App. Br. 10. Appellants argue that Chiou does not distinguish the functionality of various classes of reductants, particularly based on whether they are formaldehyde or non-formaldehyde reducing agents, and, therefore, it would not have been obvious to one of ordinary skill in the art to select an isoascorbic acid reducing agent from among the numerous reductants discloses in Chiou. Id. One of ordinary skill in the art seeking to produce polymeric polymers by emulsion polymerization as disclosed in Chiou, however, would have found it obvious to utilize any of the reducing agents that Chiou indicates are suitable for use in such a process, including isoascorbic acid. Chiou’s disclosure of a multitude of effective reducing agents does not render any particular reducing agent less obvious, and Chiou is available for all that it would have fairly suggested to a person of ordinary skill in the art at the time of Appellants’ invention. Merck & Co. v. Biocraft Labs., Inc., 874 F.2d 804, 807 (Fed. Cir. 1989) (“That the ’813 patent discloses a multitude of effective combinations does not render any particular formulation less obvious. This is especially true because the claimed composition is used for the identical purpose.”); Sinclair & Carroll Co. v. Interchemical Corp., 325 U.S. 327, 335 (1945) (“Reading a list and selecting a known compound to meet known requirements is no more ingenious than selecting the last piece to put into the last opening in a jig-saw puzzle.”); In re Leshin, 277 F.2d 197, 199 (CCPA 1960) (“Mere selection of known plastics to make a container- dispenser of a type made of plastics prior to the invention, the selection of the plastics being on the basis of suitability for the intended use, would be entirely obvious.”). Appeal 2018-005287 Application 13/589,219 14 Appellants argue that Chiou is an “inappropriate reference” because “it is entirely directed to a different and unrelated objective” than Appellants’ invention, and, therefore, “one skilled in the art seeking to solve their [Appellants’] problem would not look to augment or modify Chiou to solve their problem without undue reliance on hindsight search for certain elements of [A]ppellants’ invention.” App. Br. 9, 10. As discussed above, however, neither the particular motivation nor the avowed purpose of the inventors bears any moment on a proper analysis of whether a claimed invention would have been obvious. KSR, 550 U.S. at 419. Furthermore, the Examiner’s rejection is based upon the relied-upon disclosures of Chiou as evidenced by Density of Polymers, and the Examiner articulates a thorough, reasoned explanation grounded on sound factual findings for why the applied prior art would have suggested the aqueous composition of claim 1 to one of ordinary skill in the art at the time of Appellants’ invention. Final Act. 6–9. Consequently, the Examiner’s rejection is not based on hindsight as Appellants assert. Appellants argue that data presented in Table 2.1 of their Specification demonstrate the criticality of the styrene and alpha- methylstyrene monomer content recited in claim 1, and the criticality of forming a particulate polymer as recited in claim 1 in the presence of an isoascorbic acid reductant. App. Br. 10–11; Reply Br. 2–3. Appellants argue that the inventive aqueous compositions of Examples 2 and 3, which both included particulate polymer Sample A that contained 0.5 % by weight copolymerized alpha-methylstyrene, and was polymerized in the presence of isoascorbic acid, were “surprisingly superior” to the aqueous compositions of comparative Examples H and I, because the compositions of Examples 2 Appeal 2018-005287 Application 13/589,219 15 and 3 were free of sediment and syneresis. App. Br. 10; Reply Br. 2–3; Spec. 15, l. 1–16, l. 3; 23, l. 14–24, l. 4. The compositions of comparative Examples H and I included particulate polymer Sample B that did not contain copolymerized alpha-methylstyrene. Spec. 16, l. 20–18, l. 3. Appellants argue that the inventive aqueous compositions of Examples 2 and 3 were also “surprisingly superior” to the aqueous compositions of comparative Examples D through G, which included particulate polymer Samples C and D, which were polymerized in the presence of a sodium sulfoxylate formaldehyde reductant, rather than isoascorbic acid. App. Br. 10–11; Reply Br. 2–3; Spec. 18, l. 20–20, l. 3; 20, l. 20–22, l. 3; 23, l. 14–24, l. 4. Appellants point out that Sample C did not contain copolymerized alpha-methylstyrene, while polymer Sample D did contain copolymerized alpha-methylstyrene. Id. The burden of analyzing and explaining Specification disclosures to establish unexpected results rests with the appellants. In re Klosak, 455 F.2d 1077, 1080 (CCPA 1972) (“[T]he burden of showing unexpected results rests on he who asserts them.”). To meet this burden, the appellants must provide objective evidence demonstrating that the claimed subject matter imparts results that would have been unexpected by one of ordinary skill in the art at the time of the appellants’ invention relative to the closest prior art, which are commensurate in scope with the claimed subject matter. Id. at 1080 (“[I]t is not enough to show that results are obtained which differ from those obtained in the prior art: that difference must be shown to be an unexpected difference.”); In re Baxter Travenol Labs., 952 F.2d 388, 392 (Fed. Cir. 1991) (“[W]hen unexpected results are used as evidence of nonobviousness, the results must be shown to be unexpected compared with Appeal 2018-005287 Application 13/589,219 16 the closest prior art.”); In re Harris, 409 F.3d 1339, 1344 (Fed. Cir. 2005) (“Even assuming that the results were unexpected, Harris needed to show results covering the scope of the claimed range. Alternatively Harris needed to narrow the claims.”); In re Greenfield, 571 F.2d 1185, 1189 (CCPA 1978) (“Establishing that one (or a small number of) species gives unexpected results is inadequate proof, for ‘it is the view of this court that objective evidence of non-obviousness must be commensurate in scope with the claims which the evidence is offered to support.’” (quoting In re Tiffin, 448 F.2d 791, 792 (CCPA 1971))); On the record before us, Appellants do not meet this burden. App. Br. 6–11. First, Appellants do not explain why data for two aqueous compositions (those of Examples 2 and 3) that each include the same particulate polymer Sample A containing the same monomer (alpha- methylstyrene) at a single concentration (0.5 % by weight) are reasonably commensurate with the types and amounts of monomers recited in claim 1. Id. Second, the results obtained for the aqueous compositions of inventive Examples 2 and 3 relative to those of comparative Examples D through G do not provide a comparison to the closest prior art, because Chiou discloses use of an isoascorbic acid reducing agent. Finally, Appellants do not direct us to any persuasive evidence or averment evincing that the relied-upon results would have been unexpected by one of ordinary skill in the art at the time of their invention. Id. Appellants’ unsupported arguments to that effect cannot take the place of the evidence required to establish that the results actually would have been unexpected. In re Geisler, 116 F.3d 1465, 1470 (Fed. Cir. 1997) (quoting In re De Blauwe, 736 F.2d 699, 705 (Fed. Cir. 1984)); see also In re Pearson, 494 F.2d 1399, 1405 (CCPA 1974) Appeal 2018-005287 Application 13/589,219 17 (“Attorney’s argument in a brief cannot take the place of evidence.”). Therefore, considering the totality of the evidence relied upon in this appeal, a preponderance of the evidence weighs in favor of the Examiner’s conclusion of obviousness. We, accordingly, sustain the Examiner’s rejection of claims 1 and 3–5 under 35 U.S.C. § 103(a) as unpatentable over Chiou as evidenced by Density of Polymers. DECISION We affirm the Examiner’s rejections of claims 1 and 3–5 under 35 U.S.C. § 103(a). No time period for taking any subsequent action in connection with this appeal may be extended under 37 C.F.R. § 1.136(a)(1)(iv). AFFIRMED Copy with citationCopy as parenthetical citation