Ex Parte Olbert et alDownload PDFPatent Trial and Appeal BoardJul 25, 201612675137 (P.T.A.B. Jul. 25, 2016) Copy Citation UNITED STA TES p A TENT AND TRADEMARK OFFICE APPLICATION NO. FILING DATE FIRST NAMED INVENTOR 12/675, 137 02/25/2010 Gerhard Olbert 22850 7590 07/27/2016 OBLON, MCCLELLAND, MAIER & NEUSTADT, LLP, 1940 DUKE STREET ALEXANDRIA, VA 22314 UNITED STATES DEPARTMENT OF COMMERCE United States Patent and Trademark Office Address: COMMISSIONER FOR PATENTS P.O. Box 1450 Alexandria, Virginia 22313-1450 www .uspto.gov ATTORNEY DOCKET NO. CONFIRMATION NO. 354287USOPCT 2280 EXAMINER PUTTLITZ, KARL J ART UNIT PAPER NUMBER 1671 NOTIFICATION DATE DELIVERY MODE 07/27/2016 ELECTRONIC Please find below and/or attached an Office communication concerning this application or proceeding. The time period for reply, if any, is set in the attached communication. Notice of the Office communication was sent electronically on above-indicated "Notification Date" to the following e-mail address( es): patentdocket@oblon.com oblonpat@oblon.com ahudgens@oblon.com PTOL-90A (Rev. 04/07) UNITED STATES PATENT AND TRADEMARK OFFICE BEFORE THE PATENT TRIAL AND APPEAL BOARD Exparte GERHARD OLBERT, TORSTEN MATTKE, CARSTEN KNOESCHE, ANDREAS DAISS, and JENS DENECKE1 Appeal2014-000496 Application 12/675,137 Technology Center 1600 Before ERIC B. GRIMES, ULRIKE W. JENKS, and TIMOTHY G. MAJORS, Administrative Patent Judges. MAJORS, Administrative Patent Judge. DECISION ON APPEAL This is an appeal under 35 U.S.C. § 134 involving claims to processes for preparing isocyanates which have been rejected as obvious. We have jurisdiction under 35 U.S.C. § 6(b ). We affirm-in-part. STATEMENT OF THE CASE The present invention relates to preparing isocyanates through gas- phase phosgenation - a process of reacting phosgene and amine streams in 1 Appellants identify the Real Party in Interest as BASF SE. (Appeal Br. 1.) Appeal2014-000496 Application 12/675,137 a mixing device. (Spec. 2, 11. 31-37.) Figure 4, reproduced below, is a cross-sectional view of a mixing device for practicing the claimed processes. 5 2 1 3 . . .. 2 5 (Id. at Fig. 4.) As depicted, 1 and 2 are the amine and phosgene streams respectively, which flow through nozzles in the direction of the arrows toward a gap where the reaction takes place. (Id. at 27.) Item 3 is the reaction mixture. (Id.) Structure 5 is a "Flow Disrupter." (Id.) According to the Specification: The flow of the reactants into the mixing chamber is usually turbulent in the mixing units disclosed. The flow profile has a turbulent core flow and a wall interface layer. The wall interface layer consists of a laminar underlayer close to the wall and a laminar-turbulent transition area. In the interface layer, especially the laminar underlayer, lower speeds of flow exist than in the core. At the contact point of the reactant feeds, an area of low speed and consequently high residence time is thus formed. There may be formation and deposition of solids there. (Id. at 2, 11. 17-23.) When a flow disrupter (e.g., structure 5 from Fig. 4 above) is added, however, it "force[ s] a displacement of the flow" through the nozzle so that "interface layer thickness is reduced compared to the flow 2 Appeal2014-000496 Application 12/675,137 conditions upst[r]eam of the flow disrupter." (Id. at 3, 11. 25-26, 28-29.) A reduction in the interface layer, the Specification states, "leads to a reduced deposition tendency and shorter mixing time." (Id. at 2, 11. 27-29.) Claims 1-9 and 15-18 are on appeal. Claim 1 is illustrative: 1. A process for preparing an isocyanate by mixing and reacting in the gas phase the corresponding amine with phosgene, optionally in the presence of at least one inert medium, by contacting fluid streams of amine and phosgene and subsequently reacting them with one another, which comprises reducing the turbulent flow interface of at least one stream immediately before it is contacted with the other stream by means of at least one fluidic flow disruptor. (Appeal Br. (Claims App'x).) Claims 1-9 and 15-18 are rejected under 35 U.S.C. § 103(a) over each of Wolfert,2 Herold,3 or Jenne. 4 (Ans. 4.) DISCUSSION Issue The Examiner finds that each of Wolfert, Herold, and Jenne discloses processes for producing isocyanates in a mixing device like the claims. (Id. at 5-10.) According to the Examiner, each reference teaches structures that would disrupt fluidic flow in the amine and/or phosgene streams immediately before the streams are contacted with one another. (Id.) Based on the overlap between the prior art devices and processes, and those 2 Wolfert et al. (DE 102005042392, with reference to counterpart US 2009/0221846 Al, published Sept. 3, 2009) ("Wolfert"). 3 Herold et al. (US 2005/0113601 Al, published May 26, 2005) ("Herold"). 4 Jenne et al. (US 2003/0216597 Al, published Nov. 20, 2003) ("Jenne"). 3 Appeal2014-000496 Application 12/675,137 described in the Specification, the Examiner concludes "those of ordinary skill in the art would expect that flow would also behave the same." (Ans. 13). Thus, absent objective evidence to the contrary, the Examiner concludes the prior art devices and processes would reasonably be expected to "reduc[ e] the turbulent flow interface of at least one stream immediately before it is contacted with the other stream by means of at least one fluidic flow disrupter" as provided in the claims. (Id. at 13-14.) Appellants counter that "none of the elements in the figures in the applied prior art relied upon by the Examiner have such a function." (Reply Br. 2; see also Appeal Br. 5 ("None of the applied prior art, either individually as applied, or in combination, discloses or suggests anything with regard to the above-emphasized feature of Claim 1. ") Appellants do not contest that at least some of the structures in the prior art would, in fact, disrupt the flow of the amine or phosgene streams before the streams are reacted together. But, according to Appellants, the prior art structures disrupt flow in a different way. (See, e.g., Appeal Br. 7 ("It is not disputed that such a holder disrupts the flow, but it does so in a different way than the flow disrupter according to the invention.") Appellants contend that the "turbulent flow interface" recited in the claims is a transition area between the turbulent flow in the core of the tube/nozzle and a laminar layer closer to the walls of the tube. (Id. at 6-7.) Appellants contend "the flow disrupter according to the present invention is located along the walls of the tube, therefore, affecting exclusively the flow nearest the wall but not the flow in the center of the tube." (Id. at 7.) The prior art structures, Appellants' argument goes, do not (or do not 4 Appeal2014-000496 Application 12/675,137 sufficiently) disrupt flow near the tube walls, and so do not meet all the claim elements. (See, e.g., id. at 7 ("Although [Herold's] helical element mounted in the interior of the tube will reduce the turbulent flow interface, it will not significantly affect the laminar underlayer near to the wall, since only a flow disrupter located at the wall will disrupt flow at the wall.").) All three rejections present similar issues. Has the Examiner established a prima facie case that the claims would have been obvious over Wolfert, Herold, or Jenne? And, if so, have Appellants provided persuasive argument or objective evidence to rebut the Examiner's prima facie case? Findings of Fact FF 1. Wolfert teaches "a process for preparing isocyanates and an apparatus suitable for this purpose." (Wolfert Abstract.) An embodiment of Wolfert's apparatus is depicted in cross-section below. •:ittt·•••*'<· 5 Appeal2014-000496 Application 12/675,137 (Id. at Fig. 2.) Structures 8 and 9 are annular gaps through which phosgene streams are passed. (Id. iii! 159-160.) Structure 7 is an annular gap through which the amine stream is passed. (Id.) Structure 10 is the "reaction space" for the phosgene/amine mixture. (Id.) Wolfert teaches that the "annular gaps can have any shape" including "preferably rectangular, square, oval, ellipsoidal or circular." (Id. at iJ 48.) Wolfert also teaches "a very small transverse diffusion stretch over which the fluid elements are exchanged by turbulent and laminar diffusion and thus effect mixing is critical for mixing of the streams." (Id. at iJ 50.) Structure 13 of Fig. 2 is a narrowing of the feed line: In a preferred embodiment of the present invention, the apparatus can be configured so that the feed lines for the feed streams, preferably the amine streams, narrow at the transition to the annular gaps in the direction of the annular gaps ( 13 in Fig. 2) and the \Valls of the feed lines taper at a half opening angle, i.e., the angle between the longitudinal axis of the feed line and the narrowing wall of the feed line, of from >0° up to and including 70° .... Mixing of the various streams with little deposition of solids is achieved by means of such narrowing and angles. (Id. at iJiJ 183, 185.) FF 2. Wolfert further teaches In terms of mixing of the feed streams, an improvement in the mixing established can be achieved by installation of elements which generate a tangential velocity [i.e., a circulatory movement], for example in the feed line for the substreams .... A suitable tangential-velocity generating element would be, for example, a spirally twisted ribbon (helix) inserted in the feed line, round or annular guide plates (guide vanes) or the like. 6 Appeal2014-000496 Application 12/675,137 The effect ... is to increase the shear between flow layers of differing composition in the flow in the nozzle. (Id. at iJ67 .) FF 3. Herold teaches A process for preparing isocyanates in the gas phase, in which the mixing of the reactants and thus the reaction conditions are significantly improved by means of hydrodynamic measures such as increasing the turbulence of the feed stream in the central nozzle. As a consequence, the necessary residence time in the reactor ... and the formation of polymeric by-products which lead to caking in the reactor ... is avoided. (Herold Abstract.) The process of Herold is carried out with an apparatus as depicted in cross-section below. Fig, 1 (Id. at Fig. 1.) In this figure, A and B represent the respective amine and phosgene streams. (Id. at iii! 50, 52.) Central nozzle 5 is held in position by 7 Appeal2014-000496 Application 12/675,137 holder 4, and turbulence-generating elements 7 are located in the central nozzle through which the amine stream passes. (Id. at iJ 51.) FF 4. Herold teaches that turbulence-generating element 7 may be a round or angular oblique plate or a helical element- each of which increases the degree of turbulence in the central nozzle. (Id. at Figs. 2A, 2B, 3; iii! 37-39, 52-53; claim 4.) For example, according to Herold, the "task of the helix is to increase the degree of turbulence in the stream in the central nozzle and to twist the stream in order to utilize centrifugal effects to aid mixing of inner and outer streams." (Id. at iJ 39.) In an example, Herold teaches that the diameter of the helix and the central nozzle are the same. (Id. iJiJ 55-56.) FF 5. Jenne teaches a process and tubular reactor for forming isocyanates. (Jenne Abstract.) According to Jenne, by using "flow-related measures such as homogenization and centering of the educt streams ... formation of polymeric secondary products, which result in baked-on deposits in the reactor and a reduction in reactor service life, is consequently prevented." (Id.) Figure 1 of Jenne depicts the tubular reactor: 8 Appeal2014-000496 Application 12/675,137 (Id. at Fig. 1.) A and B are the amine and phosgene streams respectively. (Id. iii! 32, 34.) Central nozzle 3 includes flexible connecting tube 2, and is held in position by a plurality of flow homogenizers (7, 8, 9) and a flow equalizer 12 is included downstream. (Id. iii! 32-33.) Jenne teaches that the flow homogenizers "homogenize the flow velocity of the educt stream apportioned into the annular space over the entire cross-section of the annular space." (Id. at iJ 20.) Structurally, these flow homogenizers may appear as, for example, "perforated plates, screens, sintered metal, fritted elements or beds." (Id.) As to structure 2, Jenne teaches "[h]oses and preferably compensators (corrugated hoses made, for example, of stainless steel) are suitable." (Id. iJ 22.) 9 Appeal2014-000496 Application 12/675,137 Analysis A. Obviousness Over Wolfert Claim 1 We address claim 1 first and then the dependent claims to the extent they are separately argued. Appellants argue, "[ r ]egarding Wolfert et al, the figures therein do not show any flow disrupters." (App. Br. 8.) Moreover, according to Appellants, the shapes and annular gaps referenced by the Examiner "refer to the openings of the annular gaps, through which the stream is fed, but not to any flow disrupters." (Id.) Appellants also contend that Wolfert "discloses measures to reduce the turbulence of the stream" such as by including "rounded, instead of stepwise transition[ s ]" and by "installation of flow 'equalizers"' and thus the apparatus as disclosed in "does not lead to flow disruption according to the present invention." (Id. at 9.) Appellants' arguments are unpersuasive. To illustrate flow disrupters in Wolfert, the Examiner cited Figure 2, pointed to various shapes of the annular openings through which the amine or phosgene streams pass, and further cited to flow equalizers that may be installed in the feed lines. (Ans. 5-8.) Figure 2 and the related description teach that there is an angular narrowing of the amine stream at structure 13 just before mixing with the phosgene stream, which results in "[ m ]ixing the various streams with little deposition of solids." (FF 1.) Thus, Figure 2 is reasonably interpreted as showing a constriction along the walls, disrupting the amine flow and providing a beneficial reduction in solid formation as described in the Specification. (Spec. 2, 11. 31-37.) 10 Appeal2014-000496 Application 12/675,137 Moreover, contrary to Appellants' argument that Wolfert seeks to decrease turbulence, Wolfert teaches that turbulence in the feed streams may be increased by including tangential-velocity generating elements (such as a helix or annular plate). (FF 2.) The flow equalizers in Wolfert are optional (Wolfert ,-i 49) and, regardless, Appellants have not persuasively shown that such structure does not reduce the turbulent flow interface within the stream. Applying the broadest reasonable interpretation, we are not persuaded that Wolfert fails to disclose a flow disrupter within the scope of claim 1. And, on this record, we agree with the Examiner that "those of ordinary skill would expect that the reactant streams of [Wolfert] would behave as instantly claimed" and that claim 1 would have been prima facie obvious. (Ans. 9-10.) Appellants have provided insufficient persuasive evidence to rebut the Examiner's prima facie case - and, in particular, to respond to the Examiner's determination that the structures of Wolfert would be expected to reduce the turbulent flow interface in the manner claimed. In re Best, 562 F.2d 1252, 1254-55, (CCPA 1977) ("[W]here the Patent Office has reason to believe that a functional limitation asserted to be critical for establishing novelty in the claimed subject matter may, in fact, be an inherent characteristic of the prior art, it possesses the authority to require the applicant to prove that the subject matter shown to be in the prior art does not possess the characteristic relied on.") (Citation and quotation marks omitted). Attorney argument and argument focused on elements not appearing in the claims do not persuade us here that the claims are 11 Appeal2014-000496 Application 12/675,137 nonobvious. 5 Without objective, fact-based evidence showing that Wolfert's mixing apparatus would not provide the function of "reducing the turbulent flow interface of at least one stream before it is contacted with the other stream," we agree with the Examiner's findings and conclusion that claim 1 would have been obvious. Claims 8 and 9 were not argued separately and thus fall with claim 1. 37 C.F.R. § 41.37(c)(l)(iv). Claims 2, 3, and 15 Claim 2 depends from claim 1 and requires that "the fluidic flow disrupter consists in a widening of limited length." Claims 3 and 15 depend directly or indirectly from claim 2 and require that the depth d2 of the widening relative to the diameter D of the flow channel be a certain ratio (e.g., the ratio in claim 15 is "0.01to0.3:1"). (Appeal Br. (Claims App'x).) Appellants contend the prior art does not teach the claimed "widening" or the particular ratios. (App. Br. 10.) The Examiner has cited no clear disclosure in Wolfert that would teach or suggest a flow disrupter that consists in a "widening" as claimed. Nor has the Examiner provided sufficient reasoning why such a structure, including one with the particular 5 For example, Appellants contend that certain structures in the prior art are not "at the wall" and that "only a flow disrupter at the wall will disrupt the flow at the wall." (App. Br. 8.) This contention, however, lacks sufficient evidentiary support. Moreover, at least as to claim 1, there is no requirement that the flow disrupter be "at the wall" or that flow "at the wall" be disrupted. In any event, as discussed above, at least some of the flow- disrupting structures in Wolfert are "at the wall." (FF 1.) 12 Appeal2014-000496 Application 12/675,137 ratios as in claims 3 and 15, would have been obvious. We thus reverse as to claims 2, 3, and 15. Claims 4, 5, and 16 Claim 4 depends from claim 1 and requires that "the fluidic flow disrupter consists in a "constriction of limited length." Claims 5 and 16 depend directly or indirectly from claim 4 and require that the height d 1 of the constriction relative to the diameter D of the flow channel be a certain ratio (e.g., the ratio in claim 16 is "0.05 to 0.18: l "). (Appeal Br. (Claims App'x).); Appellants contend the prior art does not teach the claimed "constriction" or the particular ratios. (App. Br. 10-11.) We disagree with Appellants concerning claim 4. Figure 2 of Wolfert, including the accompanying description of the figure, shows a narrowing of the amine stream, which is a constriction of limited length. (FF 1.) We agree with Appellants, however, concerning claims 5 and 16. The Examiner has not pointed us to a sufficient teaching or suggestion in Wolfert, or provided any rationale sufficient to sustain the rejection of the claims reciting particular ratios of the constriction. We thus affirm the rejection of claim 4, but reverse as to claims 5 and 16. Claims 6 and 18 According to Appellants, the cited references do not disclose the shapes of the fluidic flow disrupter required in claim 6 (e.g., rectangles, semicircles, triangles, etc.) or claim 18 (rectangle). (App. Br. 11.) This argument is not persuasive. The Examiner has cited Fig. 2 of Wolfert and teachings that the annular gaps through which the streams flow may be any 13 Appeal2014-000496 Application 12/675,137 shape (e.g., rectangular). (Ans. 6; FF 1.) We find these disclosures sufficient to show a flow disrupter having a shape within the scope of the claims. We thus affirm the rejection of claims 6 and 18. Claims 7 and 17 According to Appellants, Wolfert does not disclose a fluidic flow disrupter that encloses an angle (phi) with the flow direction, where may be from 0 to 80° (as in claim 7) or 0° (as in claim 17). (App. Br. 11; see Spec. Fig. 7.) As to claim 7, this argument is unpersuasive. Wolfert discloses a narrowing in the wall of the feed line that defines an angle of from >0° up to an including 70° with the longitudinal axis (i.e., flow direction). (FF. 1.) The Examiner has not, however, cited to any disclosure in Wolfert showing a flow disrupter that encloses an angle of 0° with the flow direction, nor provided any rationale for why the skilled person would predictably modify Wolfert further. We thus affirm the rejection of claim 7, but reverse the rejection of claim 17. B. Obviousness Over Herold Claim 1 The Examiner rejected claims 1-9 and 15-18 over Herold. According to the Examiner, holder 4 and/or turbulence generator 7 satisfy the claimed "fluidic flow disrupter" element. (Ans. 8, 10-11.) And, like discussed above, the Examiner concludes that the skilled artisan would expect the reactant streams of Herold to behave as instantly claimed (i.e., reduce the turbulent flow interface). (Ans. 9-10.) Appellants argue that holder 4 of Herold "disrupts the flow in the center of the tube as well as at the wall ... [but] the wall interface layer is 14 Appeal2014-000496 Application 12/675,137 not disrupted, since that layer simply flows around connections of the holder to the wall and flows together behind this obstacle." (App. Br. 7.) Regarding turbulence generator 7, Appellants argue "[a]though the helical element mounted in the interior of the tube will reduce the turbulent flow interface, it will not significantly affect the laminar underlayer near to the wall, since only a flow disrupter located at the wall will disrupt flow at the wall." (Id. at 8.) The Examiner has the better position. First, Appellants provide insufficient fact-based evidence to support their contentions about how flow would behave differently in the Herold apparatus and process from what is claimed. In re Best, 562 F.2d at 1254-55. Second, because the helical element of Herold may be "at the wall," Appellants' argument that it would not disrupt the flow there is not supported. In an example, Herold teaches that the diameter of the helix and the central nozzle are the same. (FF 4.) Third, Appellants admit that the helix of Herold "will reduce the turbulent flow interface." (App. Br. 8.) That is what claim 1 requires - that it "significantly affect[ s] the laminar underlayer near to the wall" is not a requirement. (Id.) For these reasons, we affirm the rejection of claim 1 over Herold. Claims 8 and 9 were not argued separately and thus fall with claim 1. Claims 2, 3, and 15 We agree with Appellants (App. Br. 10), that the Examiner has cited no clear disclosure in Herold that would teach or suggest a flow disrupter that consists in a "widening" as in claim 2. Nor has the Examiner provided sufficient reasoning why such a structure, including one with the particular 15 Appeal2014-000496 Application 12/675,137 ratios as in claims 3 and 15, would have been obvious. We thus reverse as to claims 2, 3, and 15. Claims 4, 5, and 16 Contrary to Appellants' argument, at least the turbulence-generating element 7 of Herold can be reasonably interpreted as a "constriction" as provided in claim 4. (FF 3--4.) We agree, however, with Appellants concerning claims 5 and 16. The Examiner has not pointed us to a sufficient teaching or suggestion in Herold, or provided any rationale sufficient to sustain the rejection of the claims reciting particular ratios of the constriction. We thus affirm the rejection of claim 4, but reverse as to claims 5 and 16. Claims 6 and 18 Contrary to Appellants' argument, Herold discloses a fluidic flow disrupter having the shapes recited in claims 6 and 18. (App. Br. 11.) For example, the turbulence-generating element is an oblique plate that, in cross- sectional view, is a rectangle. (FF 4.) We thus sustain the Examiner's rejection of claims 6 and 18 over Herold. Claims 7 and 17 Herold discloses a turbulence-generating element 7, which may be a helix or round or angular oblique plate. (FF 4.) The turbulence-generating element is disposed at an angle that appears greater than 0° and less than 90° (e.g., Herold, Figs. 2A, 2B, 3), and we conclude that an angle within the scope of claim 7 would have been obvious in light of Herold's descriptions of the turbulence generating element 7. However, the Examiner has not cited to any disclosure in Herold that shows a flow disrupter that encloses an 16 Appeal2014-000496 Application 12/675,137 angle of 0°, nor provided any rationale for why the skilled person would predictably modify Herold to include such an angle. We thus affirm the rejection of claim 7, but reverse the rejection of claim 17. C. Obviousness Over Jenne Claim 1 The Examiner rejected claims 1-9 and 15-18 over Jenne. According to the Examiner, flexible connecting tube 2 and flow equalizer 12 are flow disrupters as in claim 1. (Ans. 8-9, 11.) Here again, the Examiner concludes that the skilled artisan would expect the reactant streams of Jenne to behave as instantly claimed (i.e., reduce the turbulent flow interface), and invites Appellants to provide evidence to the contrary. (Ans. 9-10, 13-14.) Appellants argue that "the flow equalizers [e.g., honeycomb and tubular structures] according to Jenne et al act exactly opposite to the flow disrupter according to the present invention." (App. Br. 9.) Appellants argue that because such equalizers orient the flow axially, they would not reduce the turbulent flow interface. (Id.) Appellants do not respond concerning the effect the flexible connecting tube 2 (e.g., corrugated stainless steel hose) would have on the amine stream flowing through the central nozzle. For reasons similar to those discussed above with respect to the rejections over Wolfert and Herold, Appellants' arguments are unpersuasive. The Examiner has provided articulated reasoning with rational underpinning to support the conclusion that the skilled person would reasonably expect the structures of Jenne to disrupt the turbulent flow interface, and Appellants have provided insufficient, fact-based evidence to show otherwise. 17 Appeal2014-000496 Application 12/675,137 We thus affirm the rejection of claim 1 over Jenne. Claims 8 and 9 were not argued separately and thus fall with claim 1. Claims 2, 3, and 15 The Examiner has cited the flexible connecting hose 2 (Fig. 1) in Jenne as satisfying the claimed "widening" as in claim 2. (Ans. 10-11.) We agree this shows a widening of limited length in the central nozzle. (FF 5.) Appellants have not persuasively shown that the Examiner's findings are incorrect. We thus affirm the rejection of claim 2 over Jenne. With respect to claims 3 and 15, however, the Examiner provided insufficient explanation to show why the particular ratios in those claims would have been obvious over Jenne. Accordingly, we reverse the rejection of claims 3 and 15. Claims 4, 5, and 16 Contrary to Appellants' argument, the flow equalizers (as well as the flow homogenizers) of Jenne can be reasonably interpreted as a "constriction" as provided in claim 4. (Ans. 10-11; FF 6.) We agree with Appellants, however, concerning claims 5 and 16. The Examiner has not pointed us to a sufficient teaching or suggestion in Jenne, or provided any rationale sufficient to sustain the rejection of the claims reciting particular ratios of the constriction. We thus affirm the rejection of claim 4, but reverse as to claims 5 and 16. Claims 6 and 18 Contrary to Appellants' argument, Jenne discloses a fluidic flow disrupter having at least one of the shapes recited in claim 6. (App. Br. 11.) The corrugations shown in flexible connecting tube 2 are semi-circular in cross-section. (FF 6; Jenne Fig. 1.) Jenne does not, however, appear to 18 Appeal2014-000496 Application 12/675,137 show any rectangular flow disrupter as recited in claim 18. We thus affirm the rejection of claim 6, but reverse the rejection of claim 18. Claims 7 and 17 The Examiner has not sufficiently explained why the angles recited in claims 7 and 17 would have been obvious over Jenne, and it is not plainly evident based on the record concerning Jenne that is before us. We thus reverse the rejections of claims 7 and 17. SUMMARY For the rejections under§ 103(a) over Wolfert: we affirm as to claims 1, 4, 6-9, and 18; we reverse as to claims 2, 3, 5, and 15-17. For the rejections under§ 103(a) over Herold: we affirm as to claims 1, 4, 6-9, and 18; we reverse as to claims 2, 3, 5, and 15-17. For the rejections under§ 103(a) over Jenne: we affirm as to claims 1, 2, 4, 6, 8, 9; we reverse as to claims 3, 5, 7, and 15-18. TIME PERIOD FOR RESPONSE No time period for taking any subsequent action in connection with this appeal may be extended under 37 C.F.R. § l.136(a). AFFIRMED-IN-PART 19 Copy with citationCopy as parenthetical citation